And in his final minutes, Beethoven's Ninth Symphony, best known for its last movement Ode to Joy, was played in line with his wishes.
He was accompanied to the Basel clinic of Swiss assisted-dying organisation Life Circle by Dr Philip Nitschke, founder of Australian right-to-die group Exit International.
Prof Goodall flew from Perth, where his daughter, son and grandchildren also live, to France last week to see relatives before arriving in Switzerland, where assisted dying is legal.
He spent his final full day exploring the botanic gardens with three of his grandchildren, who said they were proud of his bravery in the face of great public attention and were glad he would die on his own terms.
At his last press conference on Wednesday, Prof Goodall was in good spirits and sang a few bars of Ode to Joy while wearing a jumper printed with the words "Ageing Disgracefully".
But he said he would have preferred to die in Australia and previously voiced his resentment at the nation's laws, which prevented him from doing so.
"Luckily my family who are in various parts of Europe and America have rallied round and come to see me, and I welcome the opportunity to see them, which I probably wouldn't have had if I hadn't pursued this Swiss option," he told journalists.
He appeared bemused by the public interest.
"At my age, or less than my age, one wants to be free to choose the death when the death is at an appropriate time," Prof Goodall said.
His decision to seek assisted suicide came after his quality of life deteriorated and his eyesight and abilities declined.
"I no longer want to continue life," he said. "I'm happy to have a chance to end it."
Readers seeking support and information about suicide prevention can contact Lifeline on 13 11 14.
Suicide Call Back Service 1300 659 467.