Albert Ramos-Vinolas followed top seed Grigor Dimitrov out of the Grand Prix Hassan II, losing his quarter-final against Borna Coric at the ATP tournament in Morocco.
Dimitrov was defeated by veteran Tommy Robredo on Thursday, leaving Spain's Ramos-Vinolas as the highest remaining seed.
World No.24 Ramos-Vinolas was ousted by Coric 4-6 6-4 6-4 on Friday (Saturday AEST).
Third-seed Philipp Kohlschreiber advanced, though he had to come from a set down in a 3-6 7-5 6-3 win over Jan-Lennard Struff, while Robredo's run was ended in a straight-sets loss to Benoit Paire.
Jiri Vesely is the other semi-finalist following his 3-6 6-3 7-6 (7-5) triumph over Italian Paolo Lorenzi.
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